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首页> 外文期刊>The Journal of Chemical Physics >Translocation dynamics of a short polymer driven by an oscillating force
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Translocation dynamics of a short polymer driven by an oscillating force

机译:短聚合物在振荡力作用下的移位动力学

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We study the translocation dynamics of a short polymer moving in a noisy environment and driven by an oscillating force. The dynamics is numerically investigated by solving a Langevin equation in a two-dimensional domain. We consider a phenomenological cubic potential with a metastable state to model the polymer-pore interaction and the entropic free energy barrier characterizing the translocation process. The mean first translocation time of the center of inertia of polymers shows a nonmonotonic behavior, with a minimum, as a function of the number of the monomers. The dependence of the mean translocation time on the polymer chain length shows a monotonically increasing behavior for high values of the number of monomers. Moreover, the translocation time shows a minimum as a function of the frequency of the oscillating forcing field for all the polymer lengths investigated. This finding represents the evidence of the resonant activation phenomenon in the dynamics of polymer translocation, whose occurrence is maintained for different values of the noise intensity.
机译:我们研究了短聚合物在嘈杂环境中移动并由振荡力驱动的易位动力学。通过在二维域中求解Langevin方程,对动力学进行了数值研究。我们考虑具有亚稳态的现象立方势来模拟聚合物-孔相互作用和表征易位过程的熵自由能垒。聚合物的惯性中心的平均第一次移位时间显示出非单调行为,其最小程度取决于单体的数量。平均移位时间对聚合物链长的依赖性表明,对于高数量的单体,单调增加的行为。此外,对于所有研究的聚合物长度,移位时间都显示为最小的振荡强迫场频率的函数。该发现代表了聚合物易位动力学中的共振活化现象的证据,对于不同的噪声强度值,该现象得以维持。

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