A new look at the linear-modulated optically stimulated luminescence (LM-OSL) as a tool for dating and dosimetry

摘要

Optically stimulated luminescence (OSL) has been in use for dosimetry and dating in the last two decades. Since the OSL dependence on time is a featureless decaying function, a linear-modulation of the stimulating-fight intensity has been suggested [Bulur, E., 1996. An alternative technique for optically stimulated luminescence. Radiat. Meas. 26, 701-709.], which resulted in a peak-shaped curve. The properties of this curve have been studied, assuming first-, second- and general-order kinetics. in a recent paper we have shown [Chen, R., Pagonis, V., 2008. A unified presentation of thermoluminescence (TL), phosphorescence and linear-modulated OSL (LM-OSL). J. Phys. D: Appl. Phys. 41, 035102 (16).] that for general-order curves, the peak maximum cannot be expected to depend linearly on the dose of excitation. A new presentation of the LM-OSL has been suggested, in which the peak maximum is linear with the filling of trapping states, which, in turn, may be expected to be linear with the dose under appropriate conditions. In the present work, we report on results of numerical simulation of the LM-OSL using the one trap-one recombination center (OTOR) model, dealing with the traffic of carriers between one trapping state, one kind of recombination center and the conduction and valence bands during excitation and read-out, and without making any simplifying assumptions. The process during optical read-out has been followed in the simulation that consisted of the numerical solution of the relevant sets of coupled differential equations, and also by analytical treatment. Sets of parameters leading to approximately first- and second-order kinetics, and to intermediate cases, have been used and the results presented in the original and the new ways are shown. The consequences concerning dating and dosimetry are discussed.