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Hyperbranched Polymers Formed Through Self‐Condensing Vinyl Polymerization in a Continuous Stirred‐Tank Reactor (CSTR): 1. Molecular Weight Distribution

机译：通过在连续搅拌罐反应器（CSTR）中的自凝乙烯基聚合形成的超支化聚合物：1。分子量分布

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Abstract > A new Monte Carlo simulation algorithm, based on the random sampling technique, is proposed for the self‐condensing vinyl polymerization conducted in a continuous stirred‐tank reactor. In order to highlight the most fundamental aspects of the reaction system, the kinetic rate constants are assumed to be constant, and the size and structure dependence is neglected. With this ideal model, the high molecular weight (MW) tail of the weight fraction distribution W ( P ) is shown to follow the power law, W ( P )?∝? P ?α . The power exponent is represented by α?=? 1/( ηξ ) for ξ? ? ? 1/(2η), where ξ and η are defined in the text. For ξ? ≥ ? 1/(2η), the weight‐average MW cannot reach the steady state because of the power exponent with α?≤?2. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 基于随机抽样技术的新蒙特卡罗仿真算法，提出用于在连续搅拌罐反应器中进行的自冷凝乙烯基聚合。为了突出反应系统的最基本的方面，假设动力速率常数是恒定的，并且忽略尺寸和结构依赖性。利用这种理想的模型，高分子量（MW）尾部的重量分数分布 w </ i> （ p </ i> ）显示遵循权力法， w </ i> （ p </ i> ）？α？ p </ i> ？α</ sup> 。权力指数由 α？=？</ i> 1 /（ ηξ</ i> ）为了 ξ？</ i> ？＆？</ i> 1 /（2n），其中ξ和η在文本中定义。为了 ξ？</ i> ≥ ？</ i> 1 /（2η），由于α≤≤2的功率指数，重量平均MW无法达到稳态。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-24304/'>《Macromolecular theory and simulations》</a> <b style="margin: 0 2px;">|</b><span>2018年第6期</span><b style="margin: 0 2px;">|</b><span>共15页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tobita Hidetaka&option=202" target="_blank" rel="nofollow">Tobita Hidetaka;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Materials Science and EngineeringUniversity of Fukui3‐9‐1 Bunkyo Fukui 910‐8507 Japan;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1185.html" title="高分子化学（高聚物）">高分子化学（高聚物）;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hyperbranched&option=203" rel="nofollow">hyperbranched;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=molecular weight distribution&option=203" rel="nofollow">molecular weight distribution;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Monte Carlo simulation&option=203" rel="nofollow">Monte Carlo simulation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=power‐law distribution&option=203" rel="nofollow">power‐law distribution;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=theory&option=203" rel="nofollow">theory;</a> </p> <div class="translation"> 机译：超支化;分子量分布;蒙特卡罗模拟;幂律分布;理论; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704023539100.html">Hyperbranched Polymers Formed Through Self‐Condensing Vinyl Polymerization in a Continuous Stirred‐Tank Reactor (CSTR): 1. 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<b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=颜德岳&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 颜德岳</a> <span> <a href="/conference-cn-33266/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 中国化学会'99高分子学术论文报告会 </a> <span> <span> . 1999</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314851584.html">超支化聚苯乙烯基和超支化聚乙烯基聚合物的合成及性能研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=陈永盛&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 陈永盛</a> <span> . 2016</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120220187.html">在一个单一反应器中制备具有宽分子量分布的聚合物共混物的方法</a> <b>[P]</b> . <span> 中国专利： CN1210314C </span> <span> . 2005.07.13</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120104566687.html">在一个单一反应器中制备具有宽分子量分布的聚合物共混物的方法</a> <b>[P]</b> . <span> 中国专利： CN1368982A </span> <span> . 2002-09-11</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130431670111.html">Continuous polymerization process for the production of polymers having a narrow molecular weight distribution and taylor - couette - reactor for its realization</a> <b>[P]</b> . <span> 外国专利：  DE102007021012A1 </span> <span> . 2008-11-06</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：实现窄分子量分布的聚合物的连续聚合工艺及其泰勒-库埃特反应器的实现。 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130439067645.html">Continuous production of polyolefins with a bi- or multimodal molecular weight distribution comprises suspension polymerization in a series of reactors with liquid and gas recycle</a> <b>[P]</b> . <span> 外国专利：  DE102004006817A1 </span> <span> . 2005-09-01</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：连续生产具有双峰或多峰分子量分布的聚烯烃包括在一系列具有液体和气体循环的反应器中进行悬浮聚合 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130441453555.html">Process for balancing a continuous polymerization reaction and/or predicting the molecular mass distribution of the product of the reaction in one or more connected reactors comprises coupling the kinetic and thermodynamic models formed</a> <b>[P]</b> . <span> 外国专利：  DE10227270A1 </span> <span> . 2004-01-15</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在一个或多个连接的反应器中平衡连续聚合反应和/或预测反应产物的分子量分布的方法包括偶联形成的动力学模型和热力学模型 </span> </p> </li> </ul> 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