Zinc Sulfide Decorated on Nitrogen‐Doped Carbon Derived from Metal‐Organic Framework Composites for Highly Reversible Lithium‐Ion Battery Anode

Ding Hui; Huang Hsin‐Chih; Zhang Xin‐Ke; Xie Lei; Fan Jia‐Qi; Jiang Tao; Shi Dean; Ma Ning; Tsai Fang‐Chang

摘要

Abstract > On account of its low cost, non‐toxicity and high theoretical capacity, ZnS has been considered as one of the most potential anode materials for the following generation lithium‐ion batteries. However, the shortcomings that ZnS shows, such as low conductivity and large volume changes, make its wide application difficult. Herein, we combined ZnS with metal‐organic framework material (ZIF‐8) to form a carbon layer on the surface of nitrogen‐doped zinc sulfide, and obtained a new material ZnS@NC with a specific surface area of 191?m 2 ?g ?1 . The results show that the reversible specific capacity of the composite is 853?mAh?g ?1 when the current is 500?mAg ?1 , which is caused by the increase of specific capacity with nitrogen doping and the effective adjustment of the volume of the carbon layer coated on the periphery of the ZnS particles during charging and discharging process. Promisingly, the performance of ZnS@NC composite is far superior to that of the bare ZnS. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 由于其低成本，无毒和高理论能力，ZNS被认为是下列锂离子电池的最潜在的阳极材料之一。然而，ZNS所示的缺点如低导电性和大量变化，使其难以实现广泛的应用。在此，我们将ZnS与金属有机骨架材料（ZIF-8）组合以在氮气掺杂硫化锌表面上形成碳层，并获得了具有191Ω的特定表面积的新材料ZnS @ NC 2 </ sup> ？G ？1 </ sup> 。结果表明，复合材料的可逆具体容量为853？MAH？G ？1 </ sup> 当电流为500？mag ？1 </ sup> ，这是由氮掺杂的特定容量的增加引起的，并且在充电和放电过程期间涂覆在ZnS颗粒周边上的碳层的体积的有效调整。承诺，ZNS @ NC Composite的性能远远优于裸Zns。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第22期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ding Hui&option=202" target="_blank" rel="nofollow">Ding Hui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Hsin‐Chih&option=202" target="_blank" rel="nofollow">Huang Hsin‐Chih;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xin‐Ke&option=202" target="_blank" rel="nofollow">Zhang Xin‐Ke;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xie Lei&option=202" target="_blank" rel="nofollow">Xie Lei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fan Jia‐Qi&option=202" target="_blank" rel="nofollow">Fan Jia‐Qi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Tao&option=202" target="_blank" rel="nofollow">Jiang Tao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shi Dean&option=202" target="_blank" rel="nofollow">Shi Dean;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ma Ning&option=202" target="_blank" rel="nofollow">Ma Ning;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tsai Fang‐Chang&option=202" target="_blank" rel="nofollow">Tsai Fang‐Chang;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Hubei Key Laboratory of Polymer Materials Key Laboratory for the Green Preparation and Application of Functional Materials (Ministry of Education) Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials School of Materials Science;</p> <p>Department of Materials Science and EngineeringNational Taiwan University of Science and Technology10607 Taipei Taiwan;</p> <p>Hubei Key Laboratory of Polymer Materials Key Laboratory for the Green Preparation and Application of Functional Materials (Ministry of Education) Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials School of Materials Science;</p> <p>Hubei Key Laboratory of Polymer Materials Key Laboratory for the Green Preparation and Application of Functional Materials (Ministry of Education) Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials School of Materials Science;</p> <p>Hubei Key Laboratory of Polymer Materials Key Laboratory for the Green Preparation and Application of Functional Materials (Ministry of Education) Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials School of Materials Science;</p> <p>Hubei Key Laboratory of Polymer Materials Key Laboratory for the Green Preparation and Application of Functional Materials (Ministry of Education) Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials School of Materials Science;</p> <p>Hubei Key Laboratory of Polymer Materials Key Laboratory for the Green Preparation and Application of Functional Materials (Ministry of Education) Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials School of Materials Science;</p> <p>College of Chemistry and Molecular EngineeringPeking University Beijing National Laboratory for Molecular Sciences (BNLMS)Beijing 100871 P. R. China;</p> <p>Hubei Key Laboratory of Polymer Materials Key Laboratory for the Green Preparation and Application of Functional Materials (Ministry of Education) Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials School of Materials Science;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal-organic framework&option=203" rel="nofollow">metal-organic framework;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nitrogen doping&option=203" rel="nofollow">nitrogen doping;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=anode&option=203" rel="nofollow">anode;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal sulfide&option=203" rel="nofollow">metal sulfide;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium-ion battery&option=203" rel="nofollow">lithium-ion battery;</a> </p> <div class="translation"> 机译：金属有机框架;氮掺杂;阳极;金属硫化物;锂离子电池; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" 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said composites, anode for non-aqueous lithium secondary batteries which comprises said anode active material, and non-aqueous lithium secondary battery</a> <b>[P]</b> . <span> 外国专利：  US9653727B2 </span> <span> . 2017-05-16</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：金属锡-碳复合物，所述复合物的制造方法，使用所述复合物制造的非水锂二次电池用负极活性物质，构成所述负极活性物质的非水锂二次电池用负极，以及非水锂二次电池电池 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022061031','4',7,2,1,'',this,24)" class="delivery" 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