Photoassisted CO ₂2 Conversion to Fuels

机译：PhotoAssisted Co. _{2 2 转换为燃料}

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Abstract > In the context of the on‐going change from fossil fuels to renewable energy sources, there is much interest in decreasing atmospheric CO <sub>2</sub> emissions. One of the possibilities is to use CO <sub>2</sub> as feedstock of fuels and chemicals. While some catalytic CO <sub>2</sub> transformations are well known processes, they consume a considerable amount of energy to occur at significant rates and in the classical processes this energy is again produced by burning fossil fuels. For this reason, there is much current interest in developing light assisted CO <sub>2</sub> transformations, including, but not limited to, artificial photosynthesis. Rather than a comprehensive review, the present article describes a range of approaches for CO <sub>2</sub> activation based either on the direct CO <sub>2</sub> excitation with deep UV light or on the use of solar photocatalysts. Due to the extension of the field, this article is focused on two photocatalyst types, namely, TiO <sub>2</sub> containing plasmonic Au nanoparticles and graphene‐semiconductor heterojunctions. It will be emphasized the opportunities that bimetallic plasmonic nanoparticles offer to implement on commercial TiO <sub>2</sub> visible light photoresponse and selectivity towards CO <sub>2</sub> reduction. It will also be commented that adsorption of Cu <sub>2</sub> O onto defective graphene increases the photocatalytic activity of the copper semiconductor over one order of magnitude for CO <sub>2</sub> photomethanation. The last section includes some comments about possible alternatives to go beyond the current efficiencies in light assisted CO <sub>2</sub> conversion with the aim of triggering new research in the area. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 在从化石燃料到可再生能源的持续变化的背景下，对大气合作的减少有很多兴趣 <sub> 2 </ sub> 排放。其中一个可能性是使用CO <sub> 2 </ sub> 作为燃料和化学物质的原料。虽然一些催化有限公司 <sub> 2 </ sub> 转化是众所周知的过程，它们消耗了大量的能量，以在显着的速率下发生，并且在经典过程中，这种能量通过燃烧化石燃料再次产生。因此，在开发光辅助公司的情况下有很多兴趣 <sub> 2 </ sub> 转化，包括但不限于人造光合作用。本文描述了一系列CO的方法而不是全面审查 <sub> 2 </ sub> 基于直接CO的激活 <sub> 2 </ sub> 用深紫色的光线或使用太阳能光催化剂的激发。由于该领域的延伸，本文集中于两种光催化剂类型，即TiO <sub> 2 </ sub> 含有等离子体Au纳米粒子和石墨烯 - 半导体异质结。将强调有机会在商业TIO上实施的双金属等离子体纳米颗粒提供 <sub> 2 </ sub> 可见光光光响应和对CO的选择性 <sub> 2 </ sub> 减少。还将评论，吸附铜 <sub> 2 </ sub> o缺陷石墨烯增加了铜半导体的光催化活性超过一个级 <sub> 2 </ sub> 光甲烷化。最后一节包括一些关于可能的替代方案的评论，超越当前在光辅助的CO中的当前效率 <sub> 2 </ sub> 随着触发该地区新研究的目的。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16041/'>《ChemCatChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第1期</span><b style="margin: 0 2px;">|</b><span>共15页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=light-assisted CO 2 transformation&option=203" rel="nofollow">light-assisted CO 2 transformation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=deep UV photolysis&option=203" rel="nofollow">deep UV photolysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photocatalysis&option=203" rel="nofollow">photocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=graphene as photocatalyst&option=203" rel="nofollow">graphene as photocatalyst;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=gold plasmon photocatalysis&option=203" rel="nofollow">gold plasmon photocatalysis;</a> </p> <div class="translation"> 机译：光辅助CO 2转化;深紫色光解;光催化;石墨烯作为光催化剂;金等离子体光催化; 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Photoassisted CO 22 Conversion to Fuels

摘要

Photoassisted CO ₂2 Conversion to Fuels