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首页> 外文期刊>ChemCatChem >Substrate‐Assisted Deposition of Metal Oxides on Three‐Dimensional Porous Reduced Graphene Oxide Networks as Bifunctional Hybrid Electrocatalysts for the Oxygen Evolution and Oxygen Reduction Reactions
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Substrate‐Assisted Deposition of Metal Oxides on Three‐Dimensional Porous Reduced Graphene Oxide Networks as Bifunctional Hybrid Electrocatalysts for the Oxygen Evolution and Oxygen Reduction Reactions

机译：基质辅助金属氧化物沉积在三维多孔的石墨烯氧化物网络中作为双官能杂交电催化剂，用于氧气进化和氧还原反应

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Abstract > The oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) are of great importance for energy conversion processes, such as water electrolysis, metal–air batteries, and fuel cells. Herein, we report a substrate‐assisted in situ reduction method to prepare three‐dimensional reduced graphene oxide (3DRGO) networks decorated with a range of mixed cobalt oxide and nickel oxide nanosheets as a new type of bifunctional catalyst for oxygen evolution and oxygen reduction. Among the different composite catalysts, Co <sub>3</sub> O <sub>4</sub> @3DRGO showed highest catalytic activities in OER and ORR with an excellent stability. This catalyst is used to catalyze the oxygen reactions in a Zn–air battery as a proof‐of‐concept. The current results render new insights into developing low‐cost, next‐generation bifunctional catalysts for photoelectrochemical cells for energy storage and conversion. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 氧气进化反应（oer）和氧还原反应（ORR）对于能量转换方法，例如水电解，金属 - 空气电池和燃料电池具有重要意义。在此，我们报告了原位还原方法的基材，以制备具有一系列混合钴氧化物和氧化镍纳米片的三维氧化石墨烯（3DRGO）网络，作为用于氧化和氧还原的新型双官能催化剂。在不同的复合催化剂中，CO <sub> 3 </ sub> O. <sub> 4 </ sub> @ 3DRGO在OER和ORR中显示出最高的催化活性，具有出色的稳定性。该催化剂用于催化Zn-空气电池中的氧反应作为概念验证。目前的结果使新的见解为开发低成本，下一代双官能催化剂，用于光电化学电池，用于储能和转化。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16041/'>《ChemCatChem》</a> <b style="margin: 0 2px;">|</b><span>2016年第17期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Mengjia&option=202" target="_blank" rel="nofollow">Zhao Mengjia;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Xiaoxue&option=202" target="_blank" rel="nofollow">Li Xiaoxue;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Song Long&option=202" target="_blank" rel="nofollow">Song Long;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Di&option=202" target="_blank" rel="nofollow">He Di;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Zhipan&option=202" target="_blank" rel="nofollow">Zhang Zhipan;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Laboratory of Cluster Science Ministry of Education of China Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion Materials School of ChemistryBeijing Institute of TechnologyBeijing 10081 P.R. China;</p> <p>Key Laboratory of Cluster Science Ministry of Education of China Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion Materials School of ChemistryBeijing Institute of TechnologyBeijing 10081 P.R. China;</p> <p>Key Laboratory of Cluster Science Ministry of Education of China Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion Materials School of ChemistryBeijing Institute of TechnologyBeijing 10081 P.R. China;</p> <p>Key Laboratory of Cluster Science Ministry of Education of China Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion Materials School of ChemistryBeijing Institute of TechnologyBeijing 10081 P.R. China;</p> <p>Key Laboratory of Cluster Science Ministry of Education of China Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion Materials School of ChemistryBeijing Institute of TechnologyBeijing 10081 P.R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=bifunctional catalysts&option=203" rel="nofollow">bifunctional catalysts;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=cobalt&option=203" rel="nofollow">cobalt;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=graphene oxide&option=203" rel="nofollow">graphene oxide;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanostructures&option=203" rel="nofollow">nanostructures;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nickel&option=203" rel="nofollow">nickel;</a> </p> <div class="translation"> 机译：双官能催化剂;钴;石墨烯氧化物;纳米结构;镍; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022058787.html">Substrate‐Assisted Deposition of Metal Oxides on Three‐Dimensional Porous Reduced Graphene Oxide Networks as Bifunctional Hybrid Electrocatalysts 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