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首页> 外文期刊>The Journal of Chemical Physics >Hydrodynamic interactions and the diffusivity of spheroidal particles
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Hydrodynamic interactions and the diffusivity of spheroidal particles

机译:流体动力学相互作用及球芯颗粒的扩散性

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It is intuitive that the diffusivity of an isolated particle differs from those in a monodisperse suspension, in which hydrodynamic interactions between the particles are operative. Batchelor [J. Fluid Mech. 74, 1-29 (1976) and J. Fluid Mech. 131, 155-175 (1983)] calculated how hydrodynamic interactions influenced the diffusivity of a dilute suspension of spherical particles, and Russel et al. [Colloidal Dispersions (Cambridge University Press, 1991)] and Brady [J. Fluid Mech. 272, 109-134 (1994)] treated nondilute (higher particle volume fraction) suspensions. Although most particles lack perfect sphericity, little is known about the effects of hydrodynamic interactions on the diffusivity of spheroidal particles, which are the simplest shapes that can be used to model anisotropic particles. Here, we calculate the effects of hydrodynamic interactions on the translational and rotational diffusivities of spheroidal particles of arbitrary aspect ratio in dilute monodisperse suspensions. We find that the translational and rotational diffusivities of prolate spheroids are more sensitive to eccentricity than for oblate spheroids. The origin of the hydrodynamic anisotropy is that found in the stresslet field for the induced-dipole interaction. However, in the dilute limit, the effects of anisotropy are at the level of a few percent. These effects have influence on a vast range of settings, from partially frozen colloidal suspensions to the dynamics of cytoplasm. Published under license by AIP Publishing.
机译:它直观的是,分离的颗粒的扩散性与单分散悬浮液中的那些不同,其中颗粒之间的流体动力学相互作用是可操作的。 batchelor [J.流体机械。 74,1-29(1976)和J.流体机械。 131,155-175(1983)]计算流动力学相互作用如何影响球形颗粒的稀释悬浮液和russel等人的扩散性。 [胶体分散体(剑桥大学出版社,1991年)]和布拉迪[J.流体机械。 272,109-134(1994)]处理过的疏水液(更高的粒子体积分数)悬浮液。虽然大多数颗粒缺乏完美的球形,但是关于流体动力相互作用对球形颗粒的扩散率的影响很少,这是可用于模拟各向异性颗粒的最简单形状。这里,我们计算流体动力相互作用对稀单分散悬浮液任意纵横比的球形颗粒的平移和旋转扩散性的影响。我们发现,扩展和旋转扩散性与圆形球体比扁圆形球体更敏感。流体动力学各向异性的起源是在诱导 - 偶极相互作用的应力场中发现。然而,在稀释极限中,各向异性的影响均为百分点。这些效果对大量设置产生影响,从部分冷冻的胶体悬浮液到细胞质的动态。通过AIP发布在许可证下发布。

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