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Measurements of OH mole fraction and temperature up to 20 kHz by using a diode-laser-based UV absorption sensor

机译:使用基于二极管激光的紫外线吸收传感器测量OH摩尔分数和高达20 kHz的温度

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摘要

Diode-laser-based sum-frequency generation of ultraviolet (UV) radiation at 313.5 nm was utilized for high-speed absorption measurements of OH mole fraction and temperature at rates up to 20 kHz. Sensor performance was characterized over a wide range of operating conditions in a 25.4 mm path-length, steady, C_(2)H_(4)-air diffusion flame through comparisons with coherent anti-Stokes Raman spectroscopy (CARS), planar laser-induced fluorescence (PLIF), and a two-dimensional numerical simulation with detailed chemical kinetics. Experimental uncertainties of 5percent and 11percent were achieved for measured temperatures and OH mole fractions, respectively, with standard deviations of <3percent at 20 kHz and an OH detection limit of <1 part per million in a 1 m path length. After validation in a steady flame, high-speed diode-laser-based measurements of OH mole fraction and temperature were demonstrated for the first time in the unsteady exhaust of a liquid-fueled, swirl-stabilized combustor. Typical agreement of approx5percent was achieved with CARS temperature measurements at various fuel/air ratios, and sensor precision was sufficient to capture oscillations of temperature and OH mole fraction for potential use with multiparameter control strategies in combustors of practical interest.
机译:基于二极管激光的313.5 nm紫外线(UV)辐射的总频率生成用于OH摩尔分数和温度的高速吸收测量,速率高达20 kHz。通过与相干反斯托克斯拉曼光谱法(CARS),平面激光诱导的相干抗辐射比较,在25.4 mm路径长度,稳定的C_(2)H_(4)-空气扩散火焰中,在宽范围的工作条件下表征了传感器的性能荧光(PLIF),以及具有详细化学动力学的二维数值模拟。对于测得的温度和OH摩尔分数,分别获得了5%和11%的实验不确定性,在1 m的光程中,标准偏差在20 kHz时<3%,OH检测极限在<百万分之一。在稳定的火焰中进行验证后,首次在液体燃料,旋流稳定的燃烧器的不稳定排气中首次证明了基于高速基于二极管激光的OH摩尔分数和温度测量结果。在各种燃油/空气比下,通过CARS温度测量获得的典型一致性约为5%,并且传感器的精度足以捕获温度和OH摩尔分数的振荡,从而有可能与实际感兴趣的燃烧器中的多参数控制策略一起使用。

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