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Modeling of threshold and dynamics behavior of organic nanostructured lasers

机译:有机纳米结构激光器的阈值和动力学行为建模

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Organic dye molecules offer significant potential as gain media in the emerging field of optical amplification and lasing at subwavelength scales. Here, we investigate the laser dynamics in systems comprising subwavelength-structured cavities that incorporate organic dyes. To this end, we have developed a comprehensive theoretical framework able to accurately describe the interaction of organic molecules with any arbitrary photonic structure to produce single-mode lasing. The model provides explicit analytic expressions of the threshold and slope efficiency that characterize this class of lasers, and also the duration over which lasing action can be sustained before the dye photobleaches. Both the physical properties of the dyes and the optical properties of the cavities are considered. We also systematically studied the feasibility of achieving lasing action under continuous-wave excitation in optically pumped monolithic organic dye lasers. This study suggests routes to realize an organic laser that can potentially lase with a threshold of only a few W cm~(-2). Our work puts forward a theoretical formalism that could enable the advancement of nanostructured organic-based light emitting and sensing devices.
机译:有机染料分子在新兴的光放大和亚波长激光激射领域中作为增益介质具有巨大的潜力。在这里,我们研究了包含有机染料的亚波长结构腔体系统中的激光动力学。为此,我们已经开发了一个全面的理论框架,能够准确地描述有机分子与任意光子结构之间的相互作用以产生单模激光。该模型提供了表征此类激光器的阈值和斜率效率的明确解析表达式,以及在染料光漂白之前可以持续发射激光的持续时间。染料的物理性质和腔的光学性质都被考虑。我们还系统地研究了在光泵浦整体有机染料激光器中在连续波激发下实现激光作用的可行性。这项研究提出了实现有机激光的途径,该有机激光可以以仅几W cm〜(-2)的阈值发射激光。我们的工作提出了一种理论形式主义,可以促进纳米结构的有机基发光和传感设备的发展。

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