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首页> 外文期刊>Journal of Modern Optics >An effective-medium approach to the optical properties of heterogeneous materials with nonlinear properties
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An effective-medium approach to the optical properties of heterogeneous materials with nonlinear properties

机译:具有非线性特性的异质材料光学特性的有效介质方法

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We have derived an analytic approach, based on the hypothesis of the effective-medium theory, to evaluate the effective dielectric magnitudes, including the effective third order nonlinear optical susceptibility , of a heterogeneous two-component medium in which one of the components (the host matrix or the embedded particle respectively) presents nonlinear behaviour. Our formulation allows us to solve the full nonlinear problem in the whole range of concentrations without treating the nonlinear effects as a small perturbation to the linear behaviour. Therefore, it can be considered as an upper limit of the commonly used low-field nonlinear approximations for heterogeneous materials. Under certain conditions, these composites can exhibit a bistable regime that the present theory properly describes in wide ranges of the concentration, shape, wavelength, dielectric contants and intrinsic nonlinear optical susceptibility of the nonlinear component as well as in terms of the intensity of the external electric field. The present approach has been used to calculate the nonlinear optical response of Cu-Al_2O_3 nanocomposites.
机译:我们基于有效介质理论的假设推导了一种分析方法,用于评估异质两组分介质的有效介电强度,包括有效的三阶非线性光学磁化率,其中组件之一(分别是主体矩阵或嵌入的粒子)呈现非线性行为。我们的公式使我们能够解决整个浓度范围内的完全非线性问题,而无需将非线性效应视为对线性行为的微小扰动。因此,可以将其视为异质材料常用的低场非线性逼近的上限。在某些条件下,这些复合材料可表现出双稳态,本理论在非线性组分的浓度,形状,波长,介电常数和固有非线性光学磁化率以及外部强度的广泛范围内正确描述电场。本方法已用于计算Cu-Al_2O_3纳米复合材料的非线性光学响应。

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