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Lineshape theory and photon counting statistics for blinking quantum dots: a Levy walk process

机译:线形理论和量子点闪烁的光子计数统计:征程

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摘要

Motivated by recent experimental observations of power-law statistics both in spectral diffusion process and fluorescence intermittency of individual semiconductor nanocrystals (quantum dots), we consider two different but related problems: (a) a stochastic lien shape theory for the Kubo-Anderson oscillator whose frequency modulation follows power-law statistics and (b) photon counting statistics of quantum dots shows intensity fluctuation is characterized by power-law kinetics. In the first problem, we derive an analytical expression for the lienshape formula and find rich type of behaviors when compared with the standard theory. For example, new type of resonances and narrowing behavior have been found. We show that the lienshape is extremely sensitive to the way the system is prepared at time t = 0 and discuss the problem of stationarity. In the second problem, we use semiclassical photon counting statistics to characterize the fluctuation of the photon counts emitted from quantum dots. We show that the photon counting statistics problem can be mapped onto a Levy walk process. We find unusually large fluctuations in the photon counts that have not been encountered previously. In particular, we show that Mandel's Q parameter may increase in time even in the long time limit.
机译:根据最近对单个半导体纳米晶体(量子点)的光谱扩散过程和荧光间歇性进行幂律统计的实验观察,我们考虑了两个不同但相关的问题:(a)Kubo-Anderson振荡器的随机留置形状理论频率调制遵循幂律统计,并且(b)量子点的光子计数统计表明强度波动具有幂律动力学特征。在第一个问题中,我们推导了lienshape公式的解析表达式,并与标准理论相比发现了丰富的行为类型。例如,已经发现了新型的共振和变窄行为。我们表明,线性形状对于在时间t = 0时系统的制备方式极为敏感,并讨论了平稳性问题。在第二个问题中,我们使用半经典的光子计数统计量来表征从量子点发出的光子计数的波动。我们表明光子计数统计问题可以映射到征费过程。我们发现以前从未遇到过的光子计数异常大的波动。特别地,我们表明即使在很长的时间限制内,Mandel的Q参数也会随时间增加。

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