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Method for producing catalyst for dehydrogenation aromatization reaction of methane and aromatic compound

机译:甲烷和芳族化合物脱氢芳族化反应的制备催化剂的制备方法

摘要

PROBLEM TO BE SOLVED: To select a catalyst for dehydrogenation aromatization reaction of methane, a method for producing the catalyst, and an aromatic compound (particularly benzene), which achieve a high conversion rate and selectivity for the dehydrogenation aromatization reaction of methane. Provide a method of manufacturing. Tungsten carbide M-WCx (formula) doped with at least one metal M selected from the group consisting of Group 4 metals (Ti, Zr, Hf) and Group 5 metals (V, Nb, Ta). Among them, x represents a numerical value of 0.82 to 1.00.) A catalyst for dehydrogenating aromaization reaction of methane, which comprises a metallosilicate carrying (), and metallosilicate at least one metal M compound. A method for producing the catalyst, which comprises a step of forming a composite oxide of tungsten and metal M and a step of heat-treating the catalyst precursor at a temperature of 500 to 900 ° C. in the presence of methane to carbonize the catalyst precursor. A method for producing an aromatic compound that decarbides and aromaticizes methane using a catalyst. [Selection diagram] None
机译:要解决的问题:选择甲烷脱氢芳族化反应的催化剂,其制备催化剂的方法,以及芳族化合物(特别是苯),其实现高转化率和甲烷脱氢芳族化反应的选择性。提供制造方法。碳化钨M-WCX(公式)掺杂有至少一种选自组金属(Ti,Zr,HF)和第5族金属(V,Nb,Ta)的金属m。其中,X表示0.82至1.00的数值。)用于脱氢性甲烷的脱氢香味反应的催化剂,其包含载体载体(),并金属硅酸盐至少一种金属M化合物。一种制备催化剂的方法,包括形成钨和金属M的复合氧化物的步骤以及在甲烷存在下在500至900℃的温度下热处理催化剂前体的步骤,以碳化催化剂前体。一种制备芳香化合物的方法,使用催化剂替碳和芳香化甲烷。 [选择图]无

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