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Highly Confined Tunable Mid-Infrared Plasmonics in Graphene Nanoresonators

机译:石墨烯纳米谐振器中的高度可调谐可调中红外等离子体。

摘要

Single-layer graphene has been shown to have intriguing prospects as a plasmonic material, as modes having plasmon wavelengths 20 times smaller than free space (λ_p ~ λ_0/20) have been observed in the 2–6 THz range, and active graphene plasmonic devices operating in that regime have been explored. However there is great interest in understanding the properties of graphene plasmons across the infrared spectrum, especially at energies exceeding the graphene optical phonon energy. We use infrared microscopy to observe the modes of tunable plasmonic graphene nanoresonator arrays as small as 15 nm. We map the wavevector-dependent dispersion relations for graphene plasmons at mid-infrared energies from measurements of resonant frequency changes with nanoresonator width. By tuning resonator width and charge density, we probe graphene plasmons with λ_p ≤ λ_0/100 and plasmon resonances as high as 310 meV (2500 cm^–1) for 15 nm nanoresonators. Electromagnetic calculations suggest that the confined plasmonic modes have a local density of optical states more than 10^6 larger than free space and thus could strongly increase light–matter interactions at infrared energies.
机译:单层石墨烯已经显示出作为等离子体材料的诱人前景,因为在2–6 THz范围内观察到的等离子体波长比自由空间(λ_p〜λ_0/ 20)小20倍,并且有源石墨烯等离子体设备已经探索了在那种体制下运作。然而,人们对理解整个红外光谱中石墨烯等离子体激元的特性非常感兴趣,尤其是在超过石墨烯光学声子能量的能量下。我们使用红外显微镜观察可调谐等离子体等离子体石墨烯纳米谐振器阵列的模式,该阵列的尺寸小至15 nm。我们根据纳米谐振器宽度随谐振频率变化的测量结果绘制了石墨烯等离子体激元在中红外能量处与波矢有关的色散关系。通过调整谐振器的宽度和电荷密度,我们探究了λ_p≤λ_0/ 100的石墨烯等离子体激元,对于15 nm纳米谐振器,等离子体激元的谐振高达310 meV(2500 cm ^ -1)。电磁计算表明,受限的等离子体模式具有比自由空间大10 ^ 6的光学状态局部密度,因此可以极大地增加红外能量下的光-物质相互作用。

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