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Hydrodynamics and mass transfer of gas-liquid flow in micropacked bed reactors with metal foam packing

机译:金属泡沫包装微包装床反应器中气液流动流体动力学和气体流动

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摘要

Hydrodynamics and mass transfer of gas-liquid flow such as pressure drop, liquid holdup, and gas-liquid mass-transfer coefficient in micropacked bed reactors (mu PBRs) with metal foam packing are investigated with an automated platform. Parametric studies are conducted varying gas and liquid superficial velocities, pore diameters of foam packing, and liquid physical properties. Experimental results show that mu PBRs with foam packing have comparative mass transfer rate and 10 times lower pressure drop compared to the microparticles. The values of mass-transfer coefficient for three types of foam packing in mu PBRs are 1-2 orders of magnitude larger than those in large-scale trickle bed reactors with foam packing. Furthermore, empirical correlations of pressure drop, liquid holdup, and gas-liquid mass-transfer coefficient in mu PBRs with foam packing are proposed and the predicted values are found to be in good agreement with the experimental values.
机译:采用自动平台研究了微包床反应器(MU PBRS)的压降,液体储存和气液传质系数等压降,液体储存和气液传质系数的流体动力学和传质。 参数化研究是改变的气体和液体表面速度,泡沫包装的孔径和液体物理性质。 实验结果表明,与微粒相比,具有泡沫包装的Mu PBRS具有比较传质速率和10倍的压降。 MU PBRS的三种泡沫包装的质量转移系数的值比具有泡沫包装的大规模涓流床反应器中的1-2个数量级。 此外,提出了对泡沫填料的μPBRS中的压降,液体保持和气液传质系数的经验相关性,并且发现预测值与实验值良好。

著录项

  • 来源
    《AIChE Journal》 |2020年第2期|共11页
  • 作者单位

    Tsinghua Univ Dept Chem Engn State Key Lab Chem Engn Beijing 100084 Peoples R China;

    Tsinghua Univ Dept Chem Engn State Key Lab Chem Engn Beijing 100084 Peoples R China;

    Tsinghua Univ Dept Chem Engn State Key Lab Chem Engn Beijing 100084 Peoples R China;

    Tsinghua Univ Dept Chem Engn State Key Lab Chem Engn Beijing 100084 Peoples R China;

    Tsinghua Univ Dept Chem Engn State Key Lab Chem Engn Beijing 100084 Peoples R China;

  • 收录信息
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 化学工业;
  • 关键词

    foam packing; hydrodynamics; mass transfer; micropacked bed reactor;

    机译:泡沫包装;流体动力学;传质;微包床反应器;

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