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首页> 外文期刊>The Journal of Chemical Physics >Collective density fluctuations of DNA hydration water in the time-window below 1 ps
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Collective density fluctuations of DNA hydration water in the time-window below 1 ps

机译:低于1 ps的时间窗口中DNA水化水的集体密度波动

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摘要

The coherent density fluctuations propagating through DNA hydration water were studied by neutron scattering spectroscopy. Two collective modes were found to be sustained by the aqueous solvent: a propagating excitation, characterised by a speed of about 3500 ms, and another one placed at about 6 meV. These results globally agree with those previously found for the coherent excitations in bulk water, although in DNA hydration water the speed of propagating modes is definitely higher than that of the pure solvent. The short-wavelength collective excitations of DNA hydration water are reminiscent of those observed in protein hydration water and in the amorphous forms of ice.
机译:通过中子散射光谱研究了通过DNA水化水传播的相干密度波动。发现水性溶剂可维持两种集体模式:一种以约3500 ms的速度为特征的传播激发,另一种处于约6 meV。这些结果总体上与先前在散装水中的相干激发发现的结果一致,尽管在DNA水化水中,传播方式的速度肯定高于纯溶剂的传播方式。 DNA水合水的短波长集体激发让人想起在蛋白质水合水和无定形冰中观察到的激发。

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