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绿色能源与环境：英文版

绿色能源与环境：英文版

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绿色能源与环境：英文版 >2023年第5期

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  • 摘要：http://www.keaipublishing.com/gee AIMS&SCOPE Green Energy&Environment(GEE)is a peer-reviewed international and interdisciplinary research journal that focuses on all aspects of green energy and environment.This journal aims at presenting the world’s leading researches,ranging from either new or significantly improved protocols or methodologies to practical application of such fields.
  • 摘要：Energy scarcity and environmental pollution are worldwide issues which plague human development.According to projections for economic development and population growth,global energy demand is anticipated to double by 2050 and triple by2100.Better energy storage and conversion are glorious but arduous missions in the 21st century.Although the fossil fuel
  • 摘要：The aluminum-air battery is considered to be an attractive candidate as a power source for electric vehicles（EVs） because of its high theoretical energy density(8100 Wh kg-1), which is significantly greater than that of the state-of-the-art lithium-ion batteries（LIBs）. However,some technical and scientific problems preventing the large-scale development of Al-air batteries have not yet to be resolved. In this review, we present the fundamentals, challenges and the recent advances in Al-air battery technology from aluminum anode, air cathode and electrocatalysts to electrolytes and inhibitors. Firstly, the alloying of aluminum with transition metal elements is reviewed and shown to reduce the selfcorrosion of Al and improve battery performance. Additionally for the cathode, extensive studies of electrocatalytic materials for oxygen reduction/evolution including Pt and Pt alloys, nonprecious metal catalysts, and carbonaceous materials at the air cathode are highlighted.Moreover, for the electrolyte, the application of aqueous and nonaqueous electrolytes in Al-air batteries are discussed. Meanwhile, the addition of inhibitors to the electrolyte to enhance electrochemical performance is also explored. Finally, the challenges and future research directions are proposed for the further development of Al-air batteries.
  • 摘要：In this paper, we report a simple and facile self-assembly method to successfully fabricate cationic metal porphyrin-MtTMPyP（Mt= Cobalt（Ⅱ）, Manganese（Ⅲ）, or Iron（Ⅲ）; TMPyP = 5, 10, 15, 20-tetrakis（N-methylpyridinium-4-yl） porphyrin） intercalated into the layer of graphene oxide（GO） by the cooperative effects of electrostatic and π-π stacking interaction between positively charged metal porphyrin and negatively charged GO sheets. Followed by reduction with hydrazine vapor, a series of novel 2 D MtTMPyP/rGOn were fabricated. The as-prepared 2 D hybrids were fully characterized and tested as non-noble metal catalysts for oxygen reduction reaction（ORR） in an alkaline medium. The MtTMPyP/rGOn hybrids, especially CoTMPyP/rGO5, demonstrated an improved electrocatalytic activity for ORR and a number of exchanged electrons close to 4-electron reaction, increased stability and excellent tolerance to methanol, showing a potential alternative catalyst for ORR in fuel cells and air batteries.
  • 摘要：Introduction Types of paper Contributions falling into the following categories will be considered for publication:Reviews article(>10000 words),Short review(～5000 words),Feature article(>8000 words),Research paper,Short communication(～3000 words),Commentary(～1000 words),and Viewpiont(～3000 words).Please ensure that you select the
  • 摘要：Lithium-rich layered oxides(LrLOs) deliver extremely high specific capacities and are considered to be promising candidates for electric vehicle and smart grid applications. However, the application of LrLOs needs further understanding of the structural complexity and dynamic evolution of monoclinic and rhombohedral phases, in order to overcome the issues including voltage decay, poor rate capability, initial irreversible capacity loss and etc. The development of aberration correction for the transmission electron microscope and concurrent progress in electron spectroscopy, have fueled rapid progress in the understanding of the mechanism of such issues. New techniques based on the transmission electron microscope are first surveyed, and the applications of these techniques for the study of the structure, migration of transition metal, and the activation of oxygen of LrLOs are then explored in detail, with a particular focus on the mechanism of voltage decay.
  • 摘要：Engineering design of battery configurations and new battery system development are alternative approaches to achieve high performance batteries. A novel flexible and ultra-light graphite anode is fabricated by simple friction drawing on filter paper with a commercial 8 B pencil.Compared with the traditional anode using copper foil as current collector, this innovative current-collector-free design presents capacity improvement of over 200% by reducing the inert weight of the electrode. The as-prepared pencil-trace electrode exhibits excellent rate performance in potassium-ion batteries（KIBs）, significantly better than in lithium-ion batteries（LIBs）, with capacity retention of 66% for the KIB vs. 28% for the LIB from 0.1 to 0.5 A g-1. It also shows a high reversible capacity of ～230 mAh g-1 at 0.2 A g-1, 75% capacity retention over350 cycles at 0.4 A g-1and the highest rate performance（based on the total electrode weight） among graphite electrodes for K+ storage reported so far.
  • 摘要：Phosphotungstic acid is an excellent proton conductor that can be incorporated into porous supports, and nanocomposite proton exchange membrane materials made from mesoporous silica impregnated with phosphotungstic acid have been suggested for use in fuels cells operating> 100 ℃. In this work, quasielastic neutron scattering was used to study proton self-diffusion in mesoporous disordered and P6 mm symmetry silica impregnated with two concentrations of phosphotungstic acid. Overall, the silica structure had a significantly greater effect on proton conduction and diffusion than phosphotungstic acid concentration, with higher proton conduction occurring for the P6 mm symmetry silica samples. Quasielastic neutron scattering revealed two populations of protons diffusing through each sample, and that proton conduction is limited by the slower of these populations, which diffuse via a jump-diffusion mechanism. Whilst the fundamental jump-diffusion mechanism by which these slower protons moved was found to be similar for both silica supports and phosphotungstic acid concentrations, the faster diffusion occurring in P6 mm structured silica arises from a lower residence time of protons moving between sites in the jump-diffusion model, suggesting a lower energy barrier.
  • 摘要：(Quarterly)http://www.keaipublishing.com/geeAIMS&SCOPE Green Energy&Environment(GEE)is a peer-reviewed international and interdisciplinary research journal that focuses on all aspects of green energy and environment.This journal aims at presenting the world’s leading researches,ranging from either new or significantly improved protocols or methodologies to practical application of such fields.
  • 摘要：In the past decade, the aprotic lithium-oxygen（Li-O2） battery has generated a great deal of interest because theoretically it can store more energy than today’s lithium-ion batteries. Although considerable research efforts have been devoted to the R&D of this potentially disruptive technology, many scientific and engineering obstacles still remain to be addressed before a practical device could be realized. In this review, we summarize recent advances in the fundamental understanding of the O2 electrochemistry in Li-O2 batteries, including the O2 reduction to Li2O2 on discharge and the reverse Li2 O2 oxidation on recharge and factors that exert strong influences on the redox of O2/Li2O2. In addition,challenges and perspectives are also provided for the future study of Li—O2 batteries.
  • 摘要：Carbon nitride(CN_x) films supported on fluorine-doped tin oxide(FTO) glass are prepared by radio frequency magnetron sputtering, in which the film thicknesses are 90-100 nm, and the element components in the CNX films are in the range of x = 0.15-0.25. The as-prepared CN_x is for the first time used as counter electrode for dye-sensitized solar cells(DSSCs), and show a preparation-temperature dependent electrochemical performance. X-ray photoelectron spectroscopy(XPS) demonstrates that there is a higher proportion of sp~2 C=C and sp~3 C-N hybridized bonds in CN_x-500(the sample treated at 500 ℃) than in CNX-RT(the sample without a heat treatment). It is proposed that the sp~2 C=C and sp~3 C-N hybridized bonds in the CN_x films are helpful for improving the electrocatalytic activities in DSSCs. Meanwhile, Raman spectra also prove that CN_x-500 has a relatively high graphitization level that means an increasing electrical conductivity. This further explains why the sample after the heat treatment has a higher electrochemical performance in DSSCs. In addition, the as-prepared CN_x counter electrodes have a good light transmittance in the visible light region. The results are meaningful for developing low-cost metal-free transparent counter electrodes for DSSCs.
  • 摘要：The conversion of carbon dioxide into value-added products is of great industrial and environmental interest. However, as carbon dioxide is relatively stable, the input energy required for this conversion is a significant limiting factor in the system’s performance. By utilising energy from the sun, through a range of key routes, this limitation can be overcome. In this review, we present a comprehensive and critical overview of the potential routes to harvest the sun’s energy, primarily through solar-thermal technologies and plasmonic resonance effects. Focusing on the localised heating approach, this review shortlists and compares viable catalysts for the photo-thermal catalytic conversion of carbon dioxide.Further, the pathways and potential products of different carbon dioxide conversion routes are outlined with the reverse water gas shift,methanation, and methanol synthesis being of key interest. Finally, the challenges in implementing such systems and the outlook to the future are detailed.
  • 摘要：Sodium-ion batteries（SIBs） have been considered to be potential candidates for next-generation low-cost energy storage systems due to the low-cost and abundance of Na resources. However, it is a big challenge to find suitable anode materials with low-cost and good performance for the application of SIBs. Hard carbon could be a promising anode material due to high capacity and expectable low-cost if originating from biomass. Herein, we report a hard carbon material derived from abundant and abandoned biomass of sorghum stalk through a simple carbonization method. The effects of carbonization temperature on microstructure and electrochemical performance are investigated. The hard carbon carbonized at 1300 ℃ delivers the best rate capability(172 mAh g-1 at 200 mA g-1) and good cycling performance(245 mAh g-1 after 50 cycles at 20 mA g-1,96% capacity retention). This contribution provides a green route for transforming sorghum stalk waste into ''''treasure''''of promising low-cost anode material for SIBs.
  • 摘要：Metal organic frameworks(MOFs) represent a class of porous material which is formed by strong bonds between metal ions and organic linkers. By careful selection of constituents, MOFs can exhibit very high surface area, large pore volume, and excellent chemical stability.Research on synthesis, structures and properties of various MOFs has shown that they are promising materials for many applications, such as energy storage, gas storage, heterogeneous catalysis and sensing. Apart from direct use, MOFs have also been used as support substrates for nanomaterials or as sacrificial templates/precursors for preparation of various functional nanostructures. In this review, we aim to present the most recent development of MOFs as precursors for the preparation of various nanostructures and their potential applications in energy-related devices and processes. Specifically, this present survey intends to push the boundaries and covers the literatures from the year 2013 to early 2017,on supercapacitors, lithium ion batteries, electrocatalysts, photocatalyst, gas sensing, water treatment, solar cells, and carbon dioxide capture.Finally, an outlook in terms of future challenges and potential prospects towards industrial applications are also discussed.
  • 摘要：There has been a continuous need for high active, excellently durable and low-cost electrocatalysts for rechargeable zinc-air batteries. Among many low-cost metal based candidates, transition metal oxides with the CNTs composite have gained increasing attention. In this paper, the 3-D hollow sphere MnO2 nanotube-supported Co3O4 nanoparticles and its carbon nanotubes hybrid material（Co3 O4/MnO2-CNTs） have been synthesized via a simple co-precipitation method combined with post-heat treatment. The morphology and composition of the catalysts are thoroughly analyzed through SEM, TEM, TEM-mapping, XRD, EDX and XPS. In comparison with the commercial 20% Pt/C, Co3O4/MnO2,bare MnO2 nanotubes and CNTs, the hybrid Co3O4/MnO2-CNTs-350 exhibits perfect bi-functional catalytic activity toward oxygen reduction reaction and oxygen evolution reaction under alkaline condition（0.1 M KOH）. Therefore, high cell performances are achieved which result in an appropriate open circuit voltage（～1.47 V）,a high discharge peak power density(340 mW cm-2) and a large specific capacity(775 mAh g-1 at 10 mA cm-2) for the primary Zn-air battery, a small charge-discharge voltage gap and a high cycle-life(504 cycles at 10 mA cm-2 with 10 min per cycle) for the rechargeable Zn-air battery. In particular, the simple synthesis method is suitable for a large-scale production of this bifunctional material due to a green, cost effective and readily available process.
  • 摘要：Common in nature and artificial systems,quasi-liquid represents a special phase under specific conditions,where precise regulations can be conducted to accommodate various applications,such as material,biology,life and manufacture.
  • 摘要：A system of light harvesting, sensing and regulating was designed based on the photo-thermal and Seebeck effect of flexible CuO nanostructures. Cu@CuO meshes were prepared via self-oxidation of Cu mesh and utilized as the photo-thermal material. Upon irradiation by visible light, the temperature of the Cu@CuO mesh dramatically increases. The temperature difference between the irradiated and non-irradiated parts of the Cu@CuO mesh produced a measurable voltage output due to the Seebeck effect. The generated voltage was then converted into a digital signal to control a rotary neutral-density disc to filter the received light. This enabled regulation of the intensity of the incident light at a selected region. This system is cost effective and has potential applications in greenhouses, factories and smart buildings to minimize energy consumption and improve wellbeing.
  • 摘要：We here report a new CO2 capture and storage method that converts CO2 into a novel alkyl carbonate salt, denoted as CO2 SM, by a system consisting of equimolar 1,4-butanediol（BDO） and 1,2-ethylenediamine（EDA）. This novel CO2 SM was then used to prepare BaCO3 crystals through a simple and fast hydrothermal synthesis under mild conditions. The CO2 SM was both the source of CO2 and the modifier to regulate the nucleation and growth of BaCO3 crystals. The morphology of the BaCO3 crystals could be tuned from rod to shuttle by adjusting the key influencing factors, including CO2 SM concentration, mineralization temperature, and mineralization time. A possible mechanism for the synthesis of BaCO3 crystals from the CO2 SM was also presented. After the BaCO3 crystals were isolated, the filtrate of the hydrothermal reaction could be recycled to again absorb CO2 and prepare BaCO3 crystals of the same polymorph. This novel approach appears promising for preparing well-formed metal carbonates.
  • 摘要：Introduction Types of paper Contributions falling into the following categories will be considered for publication:Reviews article(>10000 words),Short review(~5000 words),Feature article(>8000 words),Research paper,Short communication(~3000 words),Commentary(~1000 words),and Viewpiont(~3000 words).Please ensure that you select the appropriate article type from the list of options when making your
  • 摘要：Photoelectrochemical(PEC) cathodic protection is considered as an environment friendly method for metals anticorrosion. In this technology, a n-type semiconductor photoanode provides the photogenerated electrons for metal to achieve cathodic protection. Comparing with traditional PEC photoanode for water splitting, it requires the photoanode providing a suitable cathodic potential for the metal, instead of pursuit ultimate photon to electric conversion efficiency, thus it is a more possible PEC technology for engineering application. To date, great efforts have been devoted to developing novel n-type semiconductors and advanced modification method to improve the performance on PEC cathodic protection metals. Herein, recent progresses in this field are summarized. We highlight the fabrication process of PEC cathodic protection thin film, various nanostructure controlling, doping, compositing methods and their operation mechanism. Finally, the current challenges and future potential works on improving the PEC cathodic protection performance are discussed.
  • 摘要：The passivation behavior of Fe in the acidic AlCl3-1-ethyl-3-methyl-imidazolium chloride（AlCl3-EMIC） ionic liquid was studied by linear sweep voltammetry and chonopotentiometry. Various approaches were used to characterize the composition and morphology of passive film formed on the Fe electrode, such as scanning electron microscopy（SEM）, Raman spectra and X-ray Photoelectron Spectroscopy（XPS）. The results showed that the critical passivation potential of Fe shifted to more negative when the molar ratio of AlCl3:EMIC changing from 2 to 1.3.A film with a light yellow color was observed on the surface of the Fe electrode after passivation. The composition of the passive film was demonstrated to be FeCl2. The passive film was composed of particulate FeCl2 with average diameter of about 500 nm. The formation of FeCl2 film was attributed to the variation of the electrolyte Lewis acidity from acidic to neutral at the interface during the dissolution process of Fe. The reason caused the variation of the electrolyte acidity was discussed.
  • 摘要：GEE is a peer-reviewed international and interdisciplinary research journal that focuses on all aspects of green energy and environment.It is inaugurated by Institute of Process Enginearing,Chinese Academy of Sciences(IPE,CAS)and co-founded by Science Press,and published quarterly by Elsevier B.V.on behalf of KeAi Communications Co.Ltd..GEE is committed to publish perspectives,ground breakings,and novel results In research fields related
  • 摘要：Rational design is important to achieve high-performance sorbents used to remove the contaminants of emerging concern（CECs） from water.However, it is hard to propose effective design guidelines due to the lack of a clear understanding of the interaction mechanisms. By means of systematic quantum chemical computations, as a case study, we investigated the interactions between zeolite X/Mn+-zeolite X(Si/Al=1,Mn+=Cu2+ and Ni2+) and three commonly used CECs（namely salicylic acid, carbamazepine and ciprofloxacin） in water to clarify the adsorption mechanisms. Our computations found that anionic salicylic acid cannot be adsorbed by neither zeolite X nor Mn+-zeolite X in neutral water due to the high electrostatic repulsion. In comparison, carbamazepine and ciprofloxacin have favorable binding energies with both zeolite X and Mn+-zeolite X, and their interactions with Mn+-zeolite X are stronger due to the joint effects of H-bond, metal complexation and electrostatic interaction. The adsorption loading of ciprofloxacin, which has a large molecular size, on Mn+-zeolite X is limited due to the steric hindrance. In general, steric hindrance, electrostatic interaction, H-bond and metal complexation are dominant factors for the examined systems in this study. Thus, for the design of high-performance absorbing materials, we should fully consider the molecular properties of pollutants（molecular size, surface electrostatic potential and atomic type, etc.）, and properly enhance the favorable effects and avoid the unfavorable factors as much as possible under the guidance of the interaction mechanisms.
  • 摘要：The phosphine-functionalized phosphonium-based ionic liquids(dppm-Q, dppe-Q, dppp-Q and dppb-Q) as the bi-functional ligands enable the efficient one-pot tandem hydroformylationeacetalization. It was found that, in dppm-Q, dppe-Q, dppp-Q and dppb-Q, the incorporated phosphino-fragments were responsible for Rh-catalyzed hydroformylation and the phosphoniums were in charge of the subsequent acetalization as the Lewis acid catalysts. Moreover, the diphosphonium-based ionic liquid of dppb-DQ could be applied as a co-solvent to immobilize the Rh/dppb-Q catalytic system with the advantages of the improved catalytic performance, the available catalyst recyclability, and the wide generality for the substrates.
  • 摘要：http://www.keaipublishing.com/gee AIMS&SCOPE Green Energy&Environment(GEE)is a peer-reviewed international and interdisciplinary research journal that focuses on all aspects of green energy and environment.This journal aims at presenting the world’s leading researches,ranging from either new or significantly improved protocols or methodologies to practical application of such fields.
  • 摘要：Activation and transformation of CO2 is one of the important issues in the field of green and sustainable chemistry. Herein, CO2 as a carbonoxygen resource was converted to CO2-polyurea with 1,6-hexanediamine through a two-step polymerization. The reaction parameters such as temperature, pressure and reaction time were examined; and several kinds of catalysts were screened in the absence and presence of NMP solvent. The formed oligomer and the final polyurea were characterized by FT-IR, VT-DRIFTS, NMR, XRD, AFM and their thermal properties were examined by TGA and DSC. It was confirmed that the final polyurea has a high thermal stability; the melting temperature is 269℃ and the decomposition temperature is above 300℃. It is a brittle polymer with a tensile strength of 18.35 MPa at break length of 1.64%. The polyurea has a stronger solvent resistance due to the ordered hydrogen bond in structure. The average molecular weight should be enhanced in the postpolymerization as the appearance, hydrogen bond intensity, crystallinity, melting point and the thermal stability changed largely compared to the oligomer. The present work provides a new kind of polyurea, it is expected to have a wide application in the field of polymer materials.
  • 摘要：Bulk heterojunction（BHJ） solar cells based on small molecules have attracted potential attention due to their promise of conveniently defined structures, high absorption coefficients, solution process-ability and easy fabrication. Three D—A—D—A type organic semiconductors（WS-31,WS-32 and WS-52） are synthesized, based on the indoline donor and benzotriazole auxiliary acceptor core, along with either bare thiophene or rigid cyclopentadithiophene as π bridge, rhodanine or carbonocyanidate as end-group. Their HOMO orbitals are delocalized throughout the whole molecules. Whereas the LUMOs are mainly localized on the acceptor part of structure, which reach up to benzothiadiazole, but no distribution on indoline donor. The first excitations for WS-31 and WS-32 are mainly originated by electron transition from HOMO to LUMO level, while for WS-52, partly related to transition between HOMO and LUMO+1 level. The small organic molecules are applied as donor components in bulk heterojunction（BHJ） organic solar cells, using PC61BM as acceptor material to check their photovoltaic performances. The BHJ solar cells based on blended layer of WS-31:PC61BM and WS-32:PC61BM processed with chloroform show overall photoelectric conversion efficiency（PCE） of 0.56% and 1.02%, respectively. WS-32 based BHJ solar cells show a higher current density originated by its relatively larger driving force of photo-induced carrier in photo-active layer to LUMO of PC61BM.
  • 摘要：We herein report a facile one-pot synthesis of MnO/N-doped carbon(N—C) composites via a sustainable cotton-template glycineenitrate combustion synthesis to yield superior anode materials for Li ion batteries. MnO nanoparticles with several nanometers were well-embedded in a porous N-doped carbon matrix. It displays the unique characteristics, including the shortened Li~+-ion transport path, increased contact areas with the electrolyte solution, inhibited volume changes and agglomeration of nanoparticles, as well as good conductivity and structural stability during the cycling process, thereby benefiting the superior cycling performance and rate capability. This favorable electrochemical performance of obtained MnO/N—C composites via a one-pot biomass-templated glycine/nitrate combustion synthesis renders the suitability as anode materials for Li-ion batteries.
  • 摘要：In this work, a new immobilization method based on dopamine（DA） self-polymerization was developed for laccase immobilization on magnetic nanoparticles（Fe3O4 NPs）. To optimize the immobilization condition including reaction pH, DA concentration and enzyme concentration, a central composite response surface method was applied. The optimal condition was determined as p H value of 5.92, laccase concentration of 0.25 mg mL-1 and DA concentration of 12.74 mg mL-1, under which a high enzyme activity recovery of 88.17% was obtained.By comparing with free laccase, the stabilities of immobilized laccase towards p H, thermostability, storage were enhanced significantly.Approximately 60% of relative activity for immobilized laccase was remained after being incubated for 6 h at 50℃, but the free laccase only remained 25%. After 40 days of storage at 4℃, the laccase immobilized by DA kept about 89% of its original activity, but the free laccase only retained 48%. After recycled 10 times, the relative activity of immobilized laccase still retained 70%. The immobilized laccase was then applied to catalyze the degradation of 4-chlorophenol（4-CP）, 86% percentage of 4-CP was removed within 2 h. After degraded 10 times, the relative activity of immobilized laccase still remained 64% of its initial activity, which exhibits an excellent reusability and operational stability.
  • 摘要：The synergistic effect of H3PMo12O40 or H3PW12O40 polyoxometalate solution（POM） and TiO2 to catalyze formic acid oxidation was investigated. Under UV irradiation, hole and electron were photogenerated by TiO2. Formic acid was oxided by the photogenerated hole and photogenerated electron was transferred to reduce polyoxometalate. With this design, formic acid can be converted into electricity in the fuel cell and hydrogen can be generated in the electrolysis cell without noble metal catalyst. Unlike other noble metal catalysts applied in the fuel cells and electrolysis cell, POM and TiO2 are stable and low cost. The maximum output power density of liquid formic acid fuel cell after 12 h UV irradiation is 5.21 mW/cm2 for phosphmolybdic acid and 22.81 m W/cm2 for phosphotungstic acid respectively. The applied potential for the hydrogen evolution is as low as 0.8 V for phosphmolybdic acid and 0.6 V for phosphotungstic acid.

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