...
首页> 外文期刊>Geoscientific Model Development Discussions >The chemistry–climate model ECHAM6.3-HAM2.3-MOZ1.0
【24h】

The chemistry–climate model ECHAM6.3-HAM2.3-MOZ1.0

机译:化学 - 气候模型ECHAM6.3-HAM2.3-MOZ1.0

获取原文
           

摘要

The chemistry–climate model ECHAM-HAMMOZ contains a detailed representation of tropospheric and stratospheric reactive chemistry and state-of-the-art parameterizations of aerosols using either a modal scheme (M7) or a bin scheme (SALSA). This article describes and evaluates the model version ECHAM6.3-HAM2.3-MOZ1.0 with a focus on the tropospheric gas-phase chemistry. A 10-year model simulation was performed to test the stability of the model and provide data for its evaluation. The comparison to observations concentrates on the year 2008 and includes total column observations of ozone and CO from IASI and OMI, Aura MLS observations of temperature, HNO3, ClO, and O3 for the evaluation of polar stratospheric processes, an ozonesonde climatology, surface ozone observations from the TOAR database, and surface CO data from the Global Atmosphere Watch network. Global budgets of ozone, OH, NOx, aerosols, clouds, and radiation are analyzed and compared to the literature. ECHAM-HAMMOZ performs well in many aspects. However, in the base simulation, lightning NOx emissions are very low, and the impact of the heterogeneous reaction of HNO3 on dust and sea salt aerosol is too strong. Sensitivity simulations with increased lightning NOx or modified heterogeneous chemistry deteriorate the comparison with observations and yield excessively large ozone budget terms and too much OH. We hypothesize that this is an impact of potential issues with tropical convection in the ECHAM model.
机译:化学气候模型ECHAM-Hammoz包含使用模态方案(M7)或肠道方案(SALSA)的对流层和平坦的反应性化学和气溶胶的最新参数的详细表示。本文介绍并评估了模型版ECHAM6.3-HAM2.3-MOZ1.0,重点是对流层气相化学。进行了10年的模型模拟以测试模型的稳定性并提供评估的数据。对2008年的观察浓缩物的比较,包括臭氧和来自IASI和OMI的总柱观察,Aura MLS的温度,HNO3,CLO和O3对极地平流层工艺的评估,臭氧源性气候,表面臭氧观察从Toar数据库,来自全球大气监视网络的Surface Co数据。分析了臭氧,哦,NOx,气溶胶,云和辐射的全球预算,并与文献相比。 Echam-Hammoz在很多方面都表现良好。然而,在基础仿真中,闪电NOx排放非常低,HNO3在灰尘和海盐气溶胶上的异质反应的影响太强。随着避雷NOx或改良的异质化学增加的敏感性模拟使得与观察结果的比较劣化,并产生过大的臭氧预算术语和太多哦。我们假设这是回波模型中热带对流的潜在问题的影响。
获取原文

客服邮箱:kefu@zhangqiaokeyan.com

京公网安备:11010802029741号 ICP备案号:京ICP备15016152号-6 六维联合信息科技 (北京) 有限公司©版权所有
  • 客服微信

  • 服务号