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Helicopter-borne observations of the continental background aerosol in combination with remote sensing and ground-based measurements

机译:大陆背景气溶胶的直升机观察与遥感和基于地面测量相结合

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This paper examines the representativeness of ground-based in situ measurements for the planetary boundary layer (PBL) and conducts a?closure study between airborne in situ and ground-based lidar measurements up to an altitude of 2300?m. The related measurements were carried out in a?field campaign within the framework of the High-Definition Clouds and Precipitation for Advancing Climate Prediction (HD(CP)2) Observational Prototype Experiment (HOPE) in September?2013 in a?rural background area of central Europe.The helicopter-borne probe ACTOS (Airborne Cloud and Turbulence Observation System) provided measurements of the aerosol particle number size distribution (PNSD), the aerosol particle number concentration (PNC), the number concentration of cloud condensation nuclei (CCN-NC), and meteorological atmospheric parameters (e.g., temperature and relative humidity). These measurements were supported by the ground-based 3+2 wavelength polarization lidar system PollyXT, which provided profiles of the particle backscatter coefficient (σbsc) for three wavelengths (355, 532, and 1064?nm). Particle extinction coefficient (σext) profiles were obtained by using a?fixed backscatter-to-extinction ratio (also lidar ratio, LR). A?new approach was used to determine profiles of CCN-NC for continental aerosol. The results of this new approach were consistent with the airborne in situ measurements within the uncertainties.In terms of representativeness, the PNSD measurements on the ground showed a?good agreement with the measurements provided with ACTOS for lower altitudes. The ground-based measurements of PNC and CCN-NC are representative of the PBL when the PBL is well mixed. Locally isolated new particle formation events on the ground or at the top of the PBL led to vertical variability in the cases presented here and ground-based measurements are not entirely representative of the PBL. Based on Mie theory (Mie, 1908), optical aerosol properties under ambient conditions for different altitudes were determined using the airborne in situ measurements and were compared with the lidar measurements. The investigation of the optical properties shows that on average the airborne-based particle light backscatter coefficient is 50.1?% smaller for 1064?nm, 27.4?% smaller for 532?nm, and 29.5?% smaller for 355?nm than the measurements of the lidar system. These results are quite promising, since in situ measurement-based Mie calculations of the particle light backscattering are scarce and the modeling is quite challenging. In contrast, for the particle light extinction coefficient we found a?good agreement. The airborne-based particle light extinction coefficient was just 8.2?% larger for 532?nm and 3?% smaller for 355?nm, for an assumed LR of 55?sr. The particle light extinction coefficient for 1064?nm was derived with a LR of 30?sr. For this wavelength, the airborne-based particle light extinction coefficient is 5.2?% smaller than the lidar measurements. For the first time, the lidar ratio of 30?sr for 1064?nm was determined on the basis of in situ measurements and the LR of 55?sr for 355 and 532?nm wavelength was reproduced for European continental aerosol on the basis of this comparison. Lidar observations and the in situ based aerosol optical properties agree within the uncertainties. However, our observations indicate that a?determination of the PNSD for a?large size range is important for a?reliable modeling of aerosol particle backscattering.
机译:本文介绍了基于地面边界层(PBL)的地面原位测量的代表性,并在原位和地面的潮端测量中进行空气传播之间的闭合研究,高度为2300Ω米。相关测量在9月份的高清云和促进气候预测(HD(CP)2)观察原型实验(HOPE)的框架内进行了现场运动,以便于9月的观察原型试验(希望)2013年?农村背景区域中欧欧洲欧洲欧洲扶手(空降云和湍流观测系统)提供了气溶胶粒子数尺寸分布(PNSD),气溶胶颗粒数浓度(PNC)的测量,云凝结核的数量浓度(CCN-NC )和气象大气参数(例如,温度和相对湿度)。这些测量由基于地基的3 + 2波长偏振激光雷达系统Pollypt支持,其为三个波长(355,532和1064Ω·nm)提供了粒子反向散射系数(ΣBSC)的轮廓。通过使用α固定的反向散射与消光比(也LiDar比率LR)获得粒子消光系数(ΣEXT)曲线。 a?新方法用于确定CCN-NC用于欧式气溶胶的轮廓。这种新方法的结果与在不确定性内的原位测量中的空中测量一致。在代表性方面,地面上的PNSD测量显示了一个良好的一致意见,该测量恰到好处为较低的海拔。当PBL良好混合时,PNC和CCN-NC的基于PNC和CCN-NC的测量值是PBL的。本地隔离在地面或PBL顶部的新颗粒形成事件导致这里呈现的病例的垂直变异性,并且基于地基测量不完全代表PBL。基于MIE理论(MIE,1908),使用空气传播测定不同高度的环境条件下的光气溶胶特性,并与LIDAR测量进行比较。光学性质的研究表明,平均空气传播的粒子光反向散射系数为50.1μm≤1064Ω·nm,27.4〜%,532·nm,29.5μm≤355Ω·nm激光雷达系统。这些结果非常有前途,因为原位测量的MIE计算粒子光反向散射的计算稀缺,建模非常具有挑战性。相比之下,对于粒子轻消隐系数,我们发现了一个良好的一致性。对于355Ω·Nm,532μm,532μm,空气中基颗粒光消光系数仅为8.2Ω··Nm,3.Δ%。衍生1064〜NM的颗粒光消光系数。对于这种波长,基于空气传播的粒子光消光系数比LIDAR测量小为5.2?%。在第一次,在原位测量的基础上确定1064℃的激光雷达比率为1064Ω·Nm,并且在此基础上为欧洲大陆气溶胶再现为35〜Sr的LR为55〜Sr。比较。 LIDAR观察和基于原位的气溶胶光学特性在不确定因素内同意。然而,我们的观察结果表明a?对于a的大尺寸范围的PNSD的测定对于a?可靠的气溶胶颗粒反向散射来说是重要的。
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