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A quasi chemistry-transport model mode for EMAC

机译:EMAC的准化学运输模型模式

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A quasi chemistry-transport model mode (QCTM) is presented for the numerical chemistry-climate simulation system ECHAM/MESSy Atmospheric Chemistry (EMAC). It allows for a quantification of chemical signals through suppression of any feedback between chemistry and dynamics. Noise would otherwise interfere too strongly. The signal is calculated from the difference of two QCTM simulations, a reference simulation and a sensitivity simulation. In order to avoid the feedbacks, the simulations adopt the following offline chemical fields: (a) offline mixing ratios of radiatively active substances enter the radiation scheme, (b) offline mixing ratios of nitric acid enter the scheme for re-partitioning and sedimentation from polar stratospheric clouds, (c) and offline methane oxidation is the exclusive source of chemical water-vapor tendencies. Any set of offline fields suffices to suppress the feedbacks, though may be inconsistent with the simulation setup. An adequate set of offline climatologies can be produced from a non-QCTM simulation using the setup of the reference simulation. Test simulations reveal the particular importance of adequate offline fields associated with (a). Inconsistencies from (b) are negligible when using adequate fields of nitric acid. Acceptably small inconsistencies come from (c), but should vanish for an adequate prescription of chemical water vapor tendencies. Toggling between QCTM and non-QCTM is done via namelist switches and does not require a source code re-compilation.
机译:针对数值化学-气候模拟系统ECHAM / MESSy大气化学(EMAC),提出了一种准化学-运输模型模式(QCTM)。它可以通过抑制化学和动力学之间的任何反馈来量化化学信号。否则,噪声将干扰太大。该信号是根据两个QCTM仿真,参考仿真和灵敏度仿真之差计算得出的。为了避免反馈,模拟采用了以下离线化学场:(a)辐射活性物质的离线混合比进入辐射方案,(b)硝酸的离线混合比进入方案以从中重新分配和沉积。极地平流层云,(c)和离线甲烷氧化是化学水蒸气趋势的唯一来源。尽管可能与仿真设置不一致,但任何一组脱机字段都足以抑制反馈。使用参考模拟的设置可以从非QCTM模拟中产生足够的离线气候。测试模拟揭示了与(a)相关的足够的离线字段的特别重要性。当使用足够的硝酸时,(b)中的不一致可以忽略不计。可接受的微小不一致性来自(c),但对于化学水蒸气趋势的适当处方应消失。 QCTM和非QCTM之间的切换是通过名称列表开关完成的,不需要重新编译源代码。

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