Screening analysis of organic micro-pollutants in road dusts from some areas in northern Vietnam: A preliminary investigation on contamination status, potential sources, human exposure, and ecological risk

摘要

Road dust samples collected from some representative areas in northern Vietnam were examined to determine the occurrence of multiple classes of organic micro-pollutants. Of 942 target compounds screened, 105 organic pollutants originating from different sources such as traffic, household, agricultural, and industrial activities, were detected at least once in our samples. Concentrations of total organic pollutants in the road dusts ranged from 7.8 to 170 mu g g(-1), with a median value of 28 mu g g(-1). Overall contamination levels were the highest in samples from an urban area, followed by those from an industrial park, a suburban area, and a rural commune, suggesting environmental impacts of urbanization and industrialization. The most predominant pollutants found in the road dusts were n-alkanes, polycyclic aromatic hydrocarbons (PAHs), and current-use chemicals such as phthalate plasticizers and pharmaceutical and personal care products (PPCPs), whereas, industrial chemicals and pesticides were detected at relatively low levels. Persons occupationally exposed to road dusts (e.g., street sweepers, vendors, and traffic policemen) were estimated to receive the highest daily intake doses of dust-bound organic pollutants that were one to two orders of magnitude greater than those received by general population. No serious human health risk associated with ingestion of contaminated road dusts was observed in this study. However, levels of some phthalates were higher than related environmental quality guidelines in terms of ecological risk. More comprehensive and detailed risk assessment of organic pollutants in road dusts should be conducted, especially for highly urbanized and industrialized areas in developing countries. (C) 2019 Elsevier Ltd. All rights reserved.