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Blinking suppression of single quantum dots in agarose gel

机译:琼脂糖凝胶中单个量子点的闪烁抑制

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摘要

Fluorescence blinking is commonly observed in single molecule/particle spectroscopy, but it is an undesirable feature in many applications. We demonstrated that single CdSe/ZnS quantum dots in agarose gel exhibited suppressed blinking behavior. In addition, the long-time exponential bending tail of the power-law blinking statistics was found to be influenced by agarose gel concentration. We suggest that electron transfer from the light state to the dark state might be blocked due to electrostatic surrounding of gel with inherent negatively charged fibers.
机译:在单分子/粒子光谱中通常观察到荧光闪烁,但是在许多应用中这是不希望有的特征。我们证明了琼脂糖凝胶中的单个CdSe / ZnS量子点表现出抑制的眨眼行为。此外,发现幂律闪烁统计数据的长时间指数弯曲尾部受到琼脂糖凝胶浓度的影响。我们认为,由于凝胶固有的带负电荷的纤维被静电包围,因此可能阻止了电子从亮态到暗态的转移。

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  • 来源
    《Applied Physicsletters》 |2010年第1期|012104.1-012104.3|共3页
  • 作者单位

    Molecular Science and Technology Program, Taiwan International Graduate Program, Academia Sinica, Taipei 10617, Taiwan and Department of Chemistry, National Tsing Hua University, Hsinchu 30013, Taiwan Research Center for Applied Sciences, Academia Sinica, Taipei 11529, Taiwan;

    Research Center for Applied Sciences, Academia Sinica, Taipei 11529, Taiwan;

    Institute of Applied Chemistry, National Chiao-Tung University, Hsinchu 30010, Taiwan;

    Research Center for Applied Sciences, Academia Sinica, Taipei 11529, Taiwan;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
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  • 正文语种 eng
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