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The roles of photo-carrier doping and driving wavelength in high harmonic generation from a semiconductor

机译:载流子掺杂和驱动波长在半导体高次谐波产生中的作用

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摘要

High-harmonic generation from gases produces attosecond bursts and enables high-harmonic spectroscopy to explore electron dynamics in atoms and molecules. Recently, high-harmonic generation from solids has been reported, resulting in novel phenomena and unique control of the emission, absent in gas-phase media. Here we investigate high harmonics from semiconductors with controllable induced photo-carrier densities, as well as the driving wavelengths. We demonstrate that the dominant generation mechanism can be identified by monitoring the variation of the harmonic spectra with the carrier density. Moreover, the harmonic spectral dependence on the driving wavelength is reported and a different dependence from the well-known one in gas-phase media is observed. Our study provides distinct control of the harmonic process from semiconductors, sheds light on the underlying mechanism and helps optimize the harmonic properties for future solid-state attosecond light sources.
机译:由气体产生的高谐波会产生阿秒脉冲,并使高谐波光谱能够探索原子和分子中的电子动力学。近来,已经报道了由固体高次谐波产生,导致气相介质中不存在的新颖现象和独特的排放控制。在这里,我们研究了具有可控制的感应光载流子密度和驱动波长的半导体产生的高次谐波。我们证明了可以通过监视谐波谱随载流子密度的变化来识别主导生成机制。此外,报告了谐波光谱对驱动波长的依赖性,并且观察到与气相介质中众所周知的依赖性不同。我们的研究为半导体的谐波过程提供了独特的控制,阐明了潜在的机理,并帮助优化了未来固态阿秒光源的谐波特性。

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