The charge and spin-dependent thermoelectric properties of different lengths of polythiophene in a molecular junction are investigated using the Bu¨ttiker probe method within Green function formalism in linear response regime. The coupling of the molecular chain to three-dimensional ferromagnetic electrodes is described by a tight-binding model for both parallel and antiparallel spin configurations. The decrease of height of transmission probability peaks and thermoelectric coeffi-cients are observed in the presence of the Bu¨ttiker probes. The reduction is more intensive in the strong dephased chains. Results show that the spin magnetothermopower is bigger than the charge magnetothermopower due to the larger differ-ence between the spin thermopowers with respect to the charge ones. In addition, we observed that the kind of carriers participating in the thermoelectric transport depends on the number of the thiophene rings.
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