The structure, magnetic properties and magnetostriction of PrxTb1-x(Fe0.6Co0.4)1.9 alloys were investigated. It was found that PrxTb1-x(Fe0.6Co0.4)1.9 alloys with x<0.4 were composed of single cubic Laves phase, while a mass of PuNi3-type phase appeared when the Pr concentration was higher than 0.4. The magnetization measurement showed that there were two different magnetic phases in Pr0.2Tb0.8(Fe0.6Co0.4)1.9 alloys. The saturation magnetostriction of Pr0.2Tb0.8(Fe0.6Co0.4)1.9 alloys at 900 kA·m-1 is 1765×10-6, which was higher than that of Tb0.27Dy0.73Fe2(1600×10-6). The spontaneous magnetostriction λ111 showed a maximum value at x=0.3.
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