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Optical spectroscopy of single self assembled quantum dots

机译:单个自组装量子点的光谱学

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摘要

We applied low temperature diffraction limited confocal optical microscopy to spatially resolve, and spectroscopically study photoluminescence from single self-assembled semiconductor quantum dots. Using selective wavelength imaging we unambiguously demonstrated that a single photoexcited quantum dot emits light in a few very narrow spectral lines. By solving numerically a many body Hamiltonian for a model quantum dot, we show that the multi-line emission spectrum is due to optical transitons between confined exciton multiplexes. We explain the measured spectrum and its dependence on the power of either cw or pulsed excitation by analytically solving the coupled rate equations for the excitation relaxation between these exciton multiplexes.
机译:我们应用了低温衍射有限共聚焦光学显微镜对空间进行分辨,并通过光谱研究了单个自组装半导体量子点的光致发光。使用选择性波长成像,我们明确地证明了单个光激发量子点在一些非常窄的光谱线中发光。通过数值求解模型量子点的多体哈密顿量,我们表明多线发射光谱是由于受限激子多路复用之间的光学跃迁引起的。通过解析求解这些激子多路复用之间的激发弛豫的耦合速率方程,我们解释了测得的光谱及其对cw或脉冲激发功率的依赖性。

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