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The Far-from- equilibrium Fluctuation of an Active Brownian Particle in an Optical Trap

机译:陷阱中活性布朗粒子的远离平衡涨落

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Active colloidal particles dissipate energies in a fashion different from Brownian particles, in that active particlesundergo directed motions characterized by a persistent length. An outstanding question, debated to date, pertains to how aquantitative and well-defined means can be established to quantify the differences between the statistical behavior of anactive particle and a passive Brownian particle. To address this question, we set out to investigate the motions of a single,induced-charge electrophoretic (ICEP) metallic Janus particles in a quadratic potential of an optical trap, by experimentsand numerical simulations. The positions of the particle under different driving forces were measured by experiments andsimulated numerically using a generalized Langevin equation. The 1-D positional histograms of the active particle,distinctively different from that of a Boltzmann distribution, reveal splitting of the positional distribution of a single peakcentered at the bottom of the well into two symmetrical peaks, whose centers move away from the center to a distanceincreasing with the driven force. Kurtosis of the particle’s spatial distribution is used as a way to quantify the deviationfrom Gaussian distribution and it was found that this deviation is a function of the particle’s rotational relaxation, thestiffness of the trap and the driving force. The temporal fluctuations of the active particle in the well are analyzed by theirpower spectral density (PSD).
机译:活性胶体粒子以不同于布朗粒子的方式耗散能量,因为该活性粒子 进行以持续长度为特征的定向运动。迄今为止,一个尚未解决的悬而未决的问题与如何解决 可以建立定量和定义明确的方法,以量化某人的统计行为之间的差异。 主动粒子和被动布朗粒子。为了解决这个问题,我们着手研究单个物体的运动, 通过实验在诱捕器的二次电位中产生感应电荷电泳(ICEP)金属Janus粒子 和数值模拟。通过实验测量了不同驱动力下颗粒的位置。 使用广义Langevin方程进行数值模拟。活性粒子的一维位置直方图 与玻尔兹曼分布的显着不同,揭示了单个峰的位置分布的分裂 以井的底部为中心,形成两个对称的峰,峰的中心偏离中心一定距离 随着驱动力的增加而增加。粒子空间分布的峰度用作量化偏差的一种方法 根据高斯分布,发现该偏差是粒子旋转弛豫的函数, 疏水阀的刚度和驱动力。井中活性颗粒的时间波动通过其波动进行分析 功率谱密度(PSD)。

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