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Remote plasmonic optical trapping on silver nanowire induced by nonlinear wave-mixing effects

机译:非线性混波效应在银纳米线上的远程等离子体光阱

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We have experimentally demonstrated remote plasmonic optical trapping on a chemically-synthesized silver nanowire (AgNW) induced by nonlinear optical effects, i.e. sum-frequency generation (SFG) and four wave-mixing (FWM). AgNWs were spin coated on a clean cover slip, and then covered with quantum dot (QD) aqueous solution. Two femtosecond IR laser pulses having different energies were focused on one end of the AgNW. SFG and FWM signal was observed at not only the excitation spot but also another end of AgNW through launching propagating plasmon modes. As results, it was found that QDs were trapped on the AgNW when two pulses were overlapped in time. QD resonance wavelength dependence on the trapping behavior indicates that trapping site on AgNW can be controlled.
机译:我们已经通过实验证明了通过非线性光学效应(即和频产生(SFG)和四波混频(FWM))诱发的化学合成银纳米线(AgNW)上的远程等离激元光学陷阱。将AgNW旋涂在干净的盖玻片上,然后用量子点(QD)水溶液覆盖。具有不同能量的两个飞秒IR激光脉冲聚焦在AgNW的一端。通过发射传播的等离子体激元模式,不仅在激发点而且在AgNW的另一端也观察到了SFG和FWM信号。结果发现,当两个脉冲在时间上重叠时,量子点被捕获在AgNW上。 QD共振波长对俘获行为的依赖性表明,可以控制AgNW上的俘获位点。

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