Influence of changes in dipole moments of a system with intramolecular coupling on the Four-Wave Mixing Signal

摘要

In this work we study the changes in the Four-Wave Mixing (FWM) signal with the modification of the permanent and transition dipolar moments of states in a coupled basis (under the inclusion of intramolecular coupling phenomenon), due to the changes in different parameters, such as coupling parameters v and Vo, strength constant A, and transition dipolar moment between the uncoupled states m_(12). Changes in the intensity and position of the resonances in the FWM signal spectra are observed with the variation in the parameters mentioned above.