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首页> 外文会议>2017 international Pittsburgh coal conference >Impact of Copper Oxidation States on the Reactivity in Partial Oxidation of Methanol
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Impact of Copper Oxidation States on the Reactivity in Partial Oxidation of Methanol

机译：铜氧化态对甲醇部分氧化反应性的影响

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摘要

1. Selectivity of partial oxidation of methanol changes with O_2/MeOH ratio and reaction time.rn2. S_(H_2) depends only on Cu oxidation state and S_(CO_2) only depends on P_(O_2).rn3. Reaction mechanisms of POM that is consistent with experimental results was proposed and verified by DFT.
机译：1.甲醇部分氧化的选择性随O_2 / MeOH比和反应时间的变化而变化。 S_（H_2）仅取决于Cu的氧化态，而S_（CO_2）仅取决于P_（O_2）.rn3。提出了与实验结果相符的POM反应机理，并通过DFT进行了验证。

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    H. Chi; C. Andolina; J. Li; M. Curnan; G. Zhou; J.Yang; G.Veser;

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    Department of Chemical and Petroleum Engineering, University of Pittsburgh;

    Department of Chemical and Petroleum Engineering, University of Pittsburgh;

    Department of Mechanical Engineering, State University of New York,Binghamton;

    Department of Chemical and Petroleum Engineering, University of Pittsburgh;

    Department of Mechanical Engineering, State University of New York,Binghamton;

    Department of Chemical and Petroleum Engineering, University of Pittsburgh,Department of Physics, University of Pittsburgh;

    Department of Chemical and Petroleum Engineering, University of Pittsburgh;

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