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Near-Completion CO-Conversion and Total H_2-Recovery by One-Step Water Gas Shift Reaction in Zeolite Membrane Reactor

机译:一步法在沸石膜反应器中完成近CO转化和总H_2回收

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摘要

1. MFI-type membranes are thermally and chemically stable for high temperature WGS reactions in coal-to-hydrogen conversion processes even with sulfur containing feeds.rn2. A membrane with relatively moderate H_2 selectivity of 40 and permeance was capable of achieving nearly complete CO conversion (>99.9%) at 500℃ and high pressure (20 bar) with catalyst load of 79g/m~2.
机译:1. MFI型膜在煤制氢转化过程中即使是含硫进料,对于高温WGS反应也具有热和化学稳定性。相对中等的H_2选择性为40且具有渗透性的膜能够在500℃和高压(20 bar)下以79 g / m〜2的催化剂负载实现近乎完全的CO转化率(> 99.9%)。

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    Department of Chemical, and Environmental Engineering University of Cincinnati, Ohio 45221, USA;

    Department of Chemical, and Environmental Engineering University of Cincinnati, Ohio 45221, USA;

    Department of Chemical, and Environmental Engineering University of Cincinnati, Ohio 45221, USA;

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